W. Zhang and F. A. DiGiano, Comparison of bacterial regrowth in distribution systems using free chlorine and chloramine: A statistical study of causative factors, Water Research, vol. hydrocarbons) or an electron donor (commonly an organic substrate) is added to reduce oxidized pollutants (nitrate, perchlorate, oxidized metals, chlorinated solvents, explosives and propellants). Answer (1 of 11): What is a heavy water nuclear reactor or a water-water nuclear reactor? Here is a part of my answer to a previous question, Why are Canadas Nuclear Reactors so safe? Molecularly imprinted nanospheres were used for the removal of micropollutants from hospital waste water [414]. 76567661, 2005. 3, no. The choice of substrate and the method of injection depend on the contaminant type and distribution in the aquifer, hydrogeology, and remediation objectives. 7, pp. 54715479, 2010. The use of deuterium is critical to the SNO function, because all three "flavours" (types) of neutrinos[92] may be detected in a third type of reaction as well, neutrino-disintegration, in which a neutrino of any type (electron, muon, or tau) scatters from a deuterium nucleus (deuteron), transferring enough energy to break up the loosely bound deuteron into a free neutron and proton via a neutral current (NC) interaction. Since most of the fuel is usually 238U, most reactor designs are based on thin fuel rods separated by moderator, allowing the neutrons to travel in the moderator before entering the fuel again. 12, pp. 107, no. S. M. Ponder, J. G. Darab, and T. E. Mallouk, Remediation of Cr(VI) and Pb(II) aqueous solutions using supported, nanoscale zero-valent iron, Environmental Science and Technology, vol. Technical problems and redesigns added about another billion to the resulting $14.4 billion price. S. D. Kelly, K. M. Kemner, G. E. Fryxell, J. Liu, S. V. Mattigod, and K. F. 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The immobilization of metallic nanoparticles in membrane has also been proved effective for degradation and dechlorination of toxic contaminants [416]. The Russian, U.S. and British navies rely on direct steam turbine propulsion, while French and Chinese ships use the turbine to generate electricity for propulsion (turbo-electric transmission). M.-J. Membrane permeability and salt rejection are shown to be effected by the number of coatings in TiO2/Al2O3 (aluminium oxide) composite ceramic membranes coated by iron oxide nanoparticles (Fe2O3) [272, 273]. 4, pp. 1, pp. 191, no. Traditional It is more resistant to neutrons, corrosion, oxidation, and high temperatures than conventional fuels. (2013) Microbiological Synthesis of 2H-Labeled Phenylalanine, Alanine, Valine, and Leucine/Isoleucine with Different Degrees of Deuterium Enrichment by the Gram-Positive Facultative Methylotrophic Bacterium revibacterium Methylicum. 1, pp. 46384642, 2006. X. M. Yan, B. Y. Shi, J. J. Lu, C. H. 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Symmetric spin and symmetric under parity. S.-H. Lee, S. Pumprueg, B. Moudgil, and W. Sigmund, Inactivation of bacterial endospores by photocatalytic nanocomposites, Colloids and Surfaces B: Biointerfaces, vol. An effort to rationalize the larger units in a fashion similar to CANDU 6 led to the CANDU 9. In 1985 what was then Ontario Hydro sparked controversy in Ontario due to its plans to sell tritium to the United States. 41, no. 12, pp. 19972009, 2003. In October 2011, the Canadian Federal Government licensed the CANDU design to Candu Energy (a wholly owned subsidiary of SNC-Lavalin), which also acquired the former reactor development and marketing division of AECL at that time. Shieh, M. Li, Y.-H. Lee, S.-D. Sheu, Y.-T. Liu, and Y.-C. Wang, Antibacterial performance of photocatalyst thin film fabricated by defection effect in visible light, Nanomedicine: Nanotechnology, Biology, and Medicine, vol. Between 1.5 to 2.1 kilograms (3.3 to 4.6lb) of tritium were recovered annually at the Darlington separation facility by 2003, of which a minor fraction was sold. The paper will briefly overview the availability and practice of different nanomaterials (particles or fibers) for removal of viruses, inorganic solutes, heavy metals, metal ions, complex organic compounds, natural organic matter, nitrate, and other pollutants present in surface water, ground water, and/or industrial water. 4, pp. These vessels have two reactors and are used in deep Arctic waters. Crespi, H., Conrad, S., Uphaus, R., Katz, J. The mechanisms involved during the bactericidal effects of Ag nanoparticles include, for example, the formation of free radicals damaging the bacterial membranes [127, 128], interactions with DNA, adhesion to cell surface altering the membrane properties, and enzyme damage [122, 129, 130]. K. Hashimoto, H. Irie, and A. 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Nevertheless, the various differences in deuterium-containing water (especially affecting the biological properties) are larger than in any other commonly occurring isotope-substituted compound because deuterium is unique among heavy stable isotopes in being twice as heavy as the lightest isotope. Get the latest news and analysis in the stock market today, including national and world stock market news, business news, financial news and more 47, no. 245265, 2009. Cost-effective nanostructured and reactive membranes are fabricated using different nanomaterials to develop more efficient water purification methods and in a study ceramic membrane of Al2O3 nanoparticles alone and doped with Fe, Mn, and La showed selectivity towards three different synthetic dyes [84]. 25, no. [35][36], The first heavy-water-moderated design in Canada was the ZEEP, which started operation just after the end of World War II. Photocatalysts like TiO2 nanoparticles are used effectively for the treatment of water contaminated with organic pollutants like polychlorinated biphenyls (PCBs), benzenes, and chlorinated alkanes [299]. 25, pp. 11831189, 2005. At that time the neutron had not yet been discovered, and the prevailing theory was that isotopes of an element differ by the existence of additional protons in the nucleus accompanied by an equal number of nuclear electrons. In October 1946, as part of the Russian Alsos, the NKVD deported to the Soviet Union from Germany the German scientists who had worked on heavy water production during the war, including Karl-Hermann Geib, the inventor of the Girdler sulfide process. 4, no. [65] It exports heavy water to countries including the Republic of Korea, China, and the United States. The detailed review has demonstrated the antibacterial efficiency of TiO2 nanoparticles, but the actual underlying mechanisms are not well defined especially under visible light. Design work continued throughout, and new design concepts were introduced that dramatically improved safety, capital costs, economics and overall performance. 1, pp. Thus semiheavy water molecules are far more common than "pure" (homoisotopic) heavy water molecules. 58865890, 2008. A. Frenot and I. S. Chronakis, Polymer nanofibers assembled by electrospinning, Current Opinion in Colloid and Interface Science, vol. 35, no. 14, no. [71] In addition, China and Argentina have agreed a contract to build a 700 MWe CANDU-6 derived reactor. The mechanisms of killing bacteria by CNTs are also due to the production of oxidative stress, disturbances to cell membrane, and so forth [233]. The projected average annual capacity factor is more than 90%. However, bioremediation processes can potentially be used to reduce the mobility of these material in the subsurface, reducing the potential for human and environmental exposure. L209L213, 2005. 1-2, pp. At the time this was considered important to the potential progress of the war. SCWRs share the steam explosion and radioactive steam release hazards of BWRs and LWRs as well as the need for extremely expensive heavy duty pressure vessels, pipes, valves, and pumps. Deuterium's absorption cross section for thermal neutrons is 0.52 millibarns (5.2 1032 m2; 1 barn = 1028 m2), while those of oxygen-16 and oxygen-17 are 0.19 and 0.24 millibarns, respectively. The stabilized nZVI particles could also be an effective way for in situ remediation of groundwater or industrial effluents [392]. Pd nanoparticles and bimetallic Pd/Au (gold) nanoparticles were used effectively for hydrodechlorination of trichloroethylene (TCE) [407, 408]. C. A. Orge, J. J. M. rfo, M. F. R. Pereira, A. M. Duarte de Farias, R. C. R. Neto, and M. A. Fraga, Ozonation of model organic compounds catalysed by nanostructured cerium oxides, Applied Catalysis B: Environmental, vol. 36, no. 7, pp. 73, no. 21012108, 2007. Heavy water was also acquired from the Cominco plant in Trail, British Columbia, Canada. 253263, 2003. 788794, 2002. J. Theron, J. 39, no. C. Fritzmann, J. Lwenberg, T. Wintgens, and T. Melin, State-of-the-art of reverse osmosis desalination, Desalination, vol. T. Urase and T. Kikuta, Separate estimation of adsorption and degradation of pharmaceutical substances and estrogens in the activated sludge process, Water Research, vol. Heavy water is used in certain types of nuclear reactors, where it acts as a neutron moderator to slow down neutrons so that they are more likely to react with the fissile uranium-235 than with uranium-238, which captures neutrons without fissioning. 1, no. 5776, pp. Typical bioremediations involves oxidations. Plants stop growing and seeds do not germinate when given only heavy water, because heavy water stops eukaryotic cell division. Though the antibacterial effect is size dependent [124], smaller Ag nanoparticles (8nm) were most effective, while larger particle size (1123nm) results in lower bactericidal activity [125]. D. M. A. Alrousan, P. S. M. Dunlop, T. A. McMurray, and J. In India, the Fast Breeder Test Reactor (FBTR) reached criticality in October 1985. 1, pp. If the temperature of the fuel bundles increases to the point where they are mechanically unstable, their horizontal layout means that they will bend under gravity, shifting the layout of the bundles and reducing the efficiency of the reactions. S. E. Coetser, R. G. M. Heath, and N. Ndombe, Diffuse pollution associated with the mining sectors in South Africa: a first-order assessment, Water Science and Technology, vol. 45914602, 2008. Section 3 discusses different types of nanomaterials focusing on membranes for treating a variety of pollutants in water/wastewater. SSV-33's hull was derived from that of the nuclear-powered Kirov-class battlecruisers with nuclear marine propulsion. Today there are 31 CANDU reactors in use around the world, and 13 "CANDU-derivatives" in India, developed from the CANDU design. 62, no. The bundles are contained in pressure tubes within a larger vessel containing additional heavy water acting purely as a moderator. Contamination from bacteria, protozoans, and viruses is possible in both ground and surface water. 227233, 2003. 18, pp. Thermal waste-burning was achieved by replacing a fraction of the uranium in the spent nuclear fuel with thorium. 606611, 2005. 42, no. 47, no. S. Zia, M. Amin, U. Manzoor, and A. S. Bhatti, Ultra-long multicolor belts and unique morphologies of tin-doped zinc oxide nanostructures, Applied Physics A: Materials Science and Processing, vol. 121131, 2007. Nanotungsten oxide and palladium-incorporated ZnO nanoparticles have shown good antibacterial properties at removal of E. coli from water [254, 255]. A. Khalil, M. A. Gondal, and M. A. Dastageer, Augmented photocatalytic activity of palladium incorporated ZnO nanoparticles in the disinfection of Escherichia coli microorganism from water, Applied Catalysis A: General, vol. This enables the use of natural unenriched uranium as the fuel. CANDU6 was essentially a version of the Pickering power plant that was redesigned to be able to be built in single-reactor units. Energy Alberta Corporation announced 27 August 2007 that they had applied for a licence to build a new nuclear plant at Lac Cardinal (30km west of the town of Peace River, Alberta), with two ACR-1000 reactors going online in 2017 producing 2.2 gigawatts (electric). Since the 1980s, dramatic improvements in LWR outage management[which?] Surface modification may lead to the enhanced photocatalytic activity of the selected compounds due to the short lifetime of reactive oxygen species and increase the affinity of modified nanomaterials towards many emerging water contaminants. 5590, pp. [9] In both these approaches, additional nutrients, vitamins, minerals, and pH buffers are added to enhance the growth and metabolism of the microorganisms. 39, no. 5, pp. The moderator vessel has a considerable thermal capability on its own and is normally kept relatively cool.[8]. Fan, and N. Xu, Effect of the surface properties on filtration performance of Al2O3-TiO2 composite membrane, Separation and Purification Technology, vol. In some cases, specialized microbial cultures are added (biostimulation). 7, pp. 39, no. 106, no. 6, no. 2-3, pp. Once HDO becomes a significant fraction of the water, heavy water becomes more prevalent as water molecules trade hydrogen atoms very frequently. This extracts a further 3040% energy from the uranium. I. C. Escobar, A. 4.3.1 Light and Heavy Water Reactors. Chlorine dioxide is expensive and results in the production of hazardous substances like chlorite and chlorate in manufacturing process. BHWP B was placed into service in 1979. 4856, 2008. 3, pp. J. Kim and J. W. Grate, Nano-biotechnology in using enzymes for environmental remediation: single-enzyme nanoparticles, in Nanotechnology and the Environment: Applications and Implications, B. Karn, T. Masciangioli, W. Zhang, V. Colvin, and P. Alivisatos, Eds., vol. K. Mulder, N. Hagens, and B. Fisher, Burning water: a comparative analysis of the energy return on water invested, Ambio, vol. 23, no. 73687372, 2000. [16], Nuclear power revolutionized the submarine, finally making it a true "underwater" vessel, rather than a "submersible" craft, which could only stay underwater for limited periods. Secure .gov websites use HTTPS. 8592, 2004. 205, no. 15, pp. It was established in 2001. 59005904, 2003. 41, no. 2, pp. [87], Romania produced heavy water at the now-decommissioned Drobeta Girdler sulfide plant for domestic and export purposes. 58, no. In the case of nuclear power, one normally includes two additional costs, the cost of permanent waste disposal, and the cost of decommissioning the plant when its useful lifetime is over. 5528, pp. M. L. Lind, D. E. Suk, T.-V. Nguyen, and E. M. V. Hoek, Tailoring the structure of thin film nanocomposite membranes to achieve seawater RO membrane performance, Environmental Science and Technology, vol. All the fuel is contained within the nuclear reactor, so no cargo or supplies space is taken up by fuel, nor is space taken up by exhaust stacks or combustion air intakes. The efficiency of NaP1 zeolites was evaluated for removal of heavy metals (Cr(III), Ni(II), Zn(II), Cu(II), and Cd(II)) from wastewater [317, 318]. [citation needed], The largest nuclear submarines ever built are the 26,500 tonne Russian Typhoon class. Fast reactors can be configured to "burn", or fission, all actinides, and given enough time, therefore drastically reduce the actinides fraction in spent nuclear fuel produced by the present world fleet of thermal neutron light water reactors, thus closing the fuel cycle. 5, pp. 17, pp. [15] TiO2 nanocomposites with mesoporous silica were also used for the treatment of aromatic pollutants [370373]. 10, pp. 17, pp. 2, pp. 959965, 1996. 364365, 2003. 2, pp. These NPPs are being used to provide operating experience and technological solutions that will be applied to the construction of the BN-1200 (OKBM Afrikantov first Gen IV reactor). 7129, pp. [citation needed], By 1962, the United States Navy had 26 operational nuclear submarines and another 30 under construction. The nanocatalyst of Ag and amidoxime fibers was used efficiently for degradation of organic dyes [404]. 64096413, 2008. 1-2, pp. The Savannah was expensive to operate since it was the only vessel using its specialized nuclear shore staff and servicing facility. Relative to Gen II-III, Gen IV reactors include: Nuclear reactors do not emit CO2 during operation, although mining and construction typically produce CO2 emissions. L. Balogh, D. R. Swanson, D. A. Tomalia, G. L. Hagnauer, and A. T. McManus, Dendrimer-Silver Complexes and Nanocomposites as Antimicrobial Agents, Nano Letters, vol. The successes at NPD and Douglas Point led to the decision to construct the first multi-unit station in Pickering, Ontario. S. Parra, S. E. Stanca, I. Guasaquillo, and K. Ravindranathan Thampi, Photocatalytic degradation of atrazine using suspended and supported TiO2, Applied Catalysis B: Environmental, vol. TiO2 nanocrystals modified with noble metal deposits and so forth were used for the degradation of methylene blue in the visible-light range [198, 365, 366]. They conclude that the concept is feasible, but further maturity of nuclear technology and the development and harmonisation of the regulatory framework would be necessary before the concept would be viable. Silver nanoparticles are derived from its salts like silver nitrate and silver chloride, and their effectiveness as biocides is documented in the literature [119123]. 1, pp. J. T. Mayo, C. Yavuz, S. Yean et al., The effect of nanocrystalline magnetite size on arsenic removal, Science and Technology of Advanced Materials, vol. 4, pp. W.-X. 15221528, 2006. P. V. Kamat, R. Huehn, and R. Nicolaescu, A sense and shoot approach for photocatalytic degradation of organic contaminants in water, Journal of Physical Chemistry B, vol. Consequently, AECL built the Bruce Heavy Water Plant (.mw-parser-output .geo-default,.mw-parser-output .geo-dms,.mw-parser-output .geo-dec{display:inline}.mw-parser-output .geo-nondefault,.mw-parser-output .geo-multi-punct{display:none}.mw-parser-output .longitude,.mw-parser-output .latitude{white-space:nowrap}441107N 812142W / 44.1854N 81.3618W / 44.1854; -81.3618 (Bruce Heavy Water Plant)),[76] which it later sold to Ontario Hydro, to ensure a reliable supply of heavy water for future power plants. H.-L. Liu and T. C.-K. Yang, Photocatalytic inactivation of Escherichia coli and Lactobacillus helveticus by ZnO and TiO2 activated with ultraviolet light, Process Biochemistry, vol. 238249, 2008. An improved antifouling performance and flux increase was also observed in silica-incorporated membranes [438]. The first such ship was USS Long Beach (CGN-9). 348354, 2006. I. M. Verstraeten, T. Heberer, J. R. Vogel, T. Speth, S. Zuehlke, and U. Duennbier, Occurrence of endocrine-disrupting and other wastewater compunds during water treatment with case studies from Lincoln, Nebraska and Berlin, Germany, Practice Periodical of Hazardous, Toxic, and Radioactive Waste Management, vol. K. Ebert, D. Fritsch, J. Koll, and C. Tjahjawiguna, Influence of inorganic fillers on the compaction behaviour of porous polymer based membranes, Journal of Membrane Science, vol. 7476, 2006. [48], Deuterium oxide is used to enhance boron neutron capture therapy, but this effect does not rely on the biological or chemical effects of deuterium, but instead on deuterium's ability to moderate (slow) neutrons without capturing them. These corrections are slightly different from the differences in p[D+] and p[OD-] of 0.44 from the corresponding ones in heavy water. The aim of the present study is to review the possible applications of the nanoparticles/fibers for the removal of pollutants from water/wastewater. Bisphosphonate-modified magnetite nanoparticles were also used to remove the radioactive metal toxins, uranium dioxide () with high efficiency from water [308]. 12831290, 2005. [32] Microorganisms can be used to reduce the toxicity and mobility of chromium by reducing hexavalent chromium, Cr(VI) to trivalent Cr (III). 102, no. 1013910145, 2009. So, further work to reduce this loss of silver ions is required for long-term control of membrane biofouling. 146, no. The Embalse Nuclear Power Station began commercial operation in January 1984. [72][73], During the second World War, the company Fosfatbolaget in Ljungaverk, Sweden, produced 2,300 liters per year of heavy water. S. V. Gaponenko, Optical Properties of Semiconductor Nanocrystals, Cambridge University Press, Cambridge, UK, 1998. 265273, 2004. Copyright 2014 M. T. Amin et al. Different types of nanomaterial like nanosorbents such as CNTs, polymeric materials (e.g., dendrimers), and zeolites have exceptional adsorption properties and are applied for removal of organics from water/wastewater [63]. 19962004, 2007. Nanoporous activated carbon fibers, prepared by electrospinning of CNTs, showed much higher organic sorption equilibrium constants for benzene, toluene, xylene, and ethylbenzene than granular activated carbon [349]. 6, pp. 42, no. [52] Genetically modified organisms are classified and controlled under the Toxic Substances Control Act of 1976 under United States Environmental Protection Agency. Tritium emissions from other CANDU plants are similarly low. The deliberately "sluggish" response of the fission process in CANDU allows controllers more time to diagnose and deal with problems. 122, no. The proposed symbol for antideuterium is D, that is, D with an overbar. Chen and C.-L. Chiang, Preparation of cotton fibers with antibacterial silver nanoparticles, Materials Letters, vol. 3, no. L. C. A. Oliveira, D. I. Petkowicz, A. Smaniotto, and S. B. C. Pergher, Magnetic zeolites: a new adsorbent for removal of metallic contaminants from water, Water Research, vol. 1-2, pp. 452456, 2008. 44, no. 5, pp. 9, pp. Nitrogen-doped ZnO and Zirconium oxide nanoparticles also have proved good antibacterial nanostructured materials [151, 256]. 9, pp. Finally, there are commercial products for efficient removal of arsenic and these include iron oxide nanoparticles and polymers and nanocrystalline titanium dioxide medium in the form of beads [331, 332]. 3-4, pp. The fuel may be dispersed in a graphite matrix. 20, no. L. Ritter, K. Solomon, P. Sibley et al., Sources, pathways, and relative risks of contaminants in surface water and groundwater: a perspective prepared for the Walkerton inquiry, Journal of Toxicology and Environmental HealthPart A, vol. TiO2 photocatalysts and metallic and metal-oxide nanoparticles are among the most promising nanomaterials with antimicrobial properties. 243, no. In a study, TiO2 nanocomposites with multiwalled CNTs showed the complete inactivation of bacterial endospores (Bacillus cereus), compared to commercial TiO2 nanoparticles [214]. 8, pp. 15, pp. Different isotopes of chemical elements have slightly different chemical behaviors, but for most elements the differences are far too small to have a biological effect. CANDU was designed for natural uranium with only 0.7%235U, so reprocessed uranium with 0.9%235U is a comparatively rich fuel. The next-generation Advanced CANDU reactor (ACR) mitigates these disadvantages by having light-water coolant and using a more compact core with less moderator. H. Hildebrand, K. Mackenzie, and F.-D. Kopinke, Novel nano-catalysts for wastewater treatment, Global Nest Journal, vol. Early thermal spectrum concepts and many current ones rely on uranium tetrafluoride (UF4) or thorium tetrafluoride (ThF4), dissolved in molten fluoride salt. HTGR runs on TRi-structural ISOtropic (TRISO) particle fuel. H.-L. Lien and W.-X. The Bruce Heavy Water Plant (BHWP) in Ontario was the world's largest heavy water production plant with a capacity of 1600 tonnes per year at its peak (800 tonnes per year per full plant, two fully operational plants at its peak). 109127, 2005. The quantity of heavy water involved was far below levels that could induce heavy water toxicity, but several employees received elevated radiation doses from tritium and neutron-activated chemicals in the water. 217225, 2008. 389404, 2003. In part due to allied sabotage and commando raids on Norsk Hydro (then the world's largest producer of heavy water) as well as the aforementioned infighting, the German nuclear program never managed to assemble enough uranium and heavy water in one place to achieve criticality despite possessing enough of both by the end of the war. 68, pp. Of the 29 commercial CANDU reactors built, 22 are in Ontario. 107-108, pp. This plot allows samples of precipitation-originated water to be identified along with general information about the climate in which it originated. 399403, 2005. K. Zhang, K. C. Kemp, and V. Chandra, Homogeneous anchoring of TiO2 nanoparticles on graphene sheets for waste water treatment, Materials Letters, vol. [70], CANDU Energy is continuing marketing efforts in China. S. Iwamoto, W. Tanakulrungsank, M. Inoue, K. Kagawa, and P. Praserthdam, Synthesis of large-surface area silica-modified titania ultrafine particles by the glycothermal method, Journal of Materials Science Letters, vol. India is one of the world's largest producers of heavy water through its Heavy Water Board. 6, no. Deuterium is a hydrogen isotope with a nucleus containing a neutron and a proton; the nucleus of a protium (normal hydrogen) atom consists of just a proton. The rapidly increasing population, depleting water resources, and climate change resulting in prolonged droughts and floods have rendered drinking water a competitive resource in many parts of the world. 10691077, 2004. Its boiling point is higher as compared to the ordinary water. Finally, the addition of metal oxide nanoparticles including silica, TiO2, alumina, and zeolites to polymeric ultrafiltration membranes has helped reducing fouling [441445]. 5, pp. J. Xu, L. Bachas, and D. Bhattacharyya, Synthesis of nanostructured bimetallic particles in polyligand-functionalized membranes for remediation applications, in Nanotechnology Applications for Clean Water, N. Savage, M. Diallo, J. Duncan, A. The toxicity of the standard chlorine chemical disinfection in addition to the carcinogenic and very harmful by-products formation is already mentioned. B. Hughes, and M. S. Wong, Designing Pd-on-Au bimetallic nanoparticle catalysts for trichloroethene hydrodechlorination, Environmental Science and Technology, vol. 65, no. 13781383, 2005. J. M. Macak, M. Zlamal, J. Krysa, and P. Schmuki, Self-organized TiO2 nanotube layers as highly efficient photocatalysts, Small, vol. 24, pp. Metal-doped TiO2 nanoparticles, sulfur, and iron in couple of studies have shown strong antibacterial effects against E. coli [203, 204]. A. F. C. Campos, R. Aquino, T. A. P. G. Cotta, F. A. Tourinho, and J. Depeyrot, Using speciation diagrams to improve synthesis of magnetic nanosorbents for environmental applications, Bulletin of Materials Science, vol.
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